How to contact a network provider regarding abuse?

I need some advice on abuse reporting as I am new to this abuse reporting scenario. I know the typical emailing the provider about abuse thing, but the Email given on IRT WHOIS is a gmail account. On top of that:

552-5.2.2 The recipient's inbox is out of storage space and inactive.

and now I am out of options regarding what I should do about it? The network in question is aggressively bruteforcing all IP addresses in our subnets and I am thinking of calling them on the phone number given in IRT WHOIS. Obviously this isn’t affecting our network much but that constant 10Mbps usage is bugging me.

Any recommendation or advice?

At a certain point you assume the network owner to be criminal and simply block their whole network. If they’re not accepting abuse complaints, that’s a pretty good reason to.